|
|
The development of magnetic behavior in the PrNi1-xCuxAl compounds
Fikáček, Jan ; Javorský, Pavel (advisor) ; Prchal, Jiří (referee)
In the present work we studied magnetic properties of the substituted PrNi1-xCuxAl series. A very interesting behavior had been reported in the previously studied systems with the same substitution, but with different rare earths contained, e.g. loss of long range order for certain concentrations of copper. We prepared polycrystalline samples of the PrNi1-xCuxAl (x = 0.1 - 0.9, 9 different stoichiometries) and measured them using X-ray diffraction, specific heat, magnetization and AC susceptibility. Additionally, powder neutron diffraction measurement on PrNi0.2Cu0.8Al sample was performed in ILL (Institut Laue Langevin) in Grenoble. Results of measurements on these compounds show on the presence of a long order in case of compounds with x = 0.1 - 0.4 below the ordering temperatures in the range of 3.4 - 5 K. Measurements of AC susceptibility and neutron diffraction revealed the loss of long range order in the rest of the series. In these compounds, the development of a spin glass state occurs below the temperatures between 3.4 and 4.5 K.
|
|
|
The development of magnetic behavior in the PrNi1-xCuxAl compounds
Fikáček, Jan
Title: The development of magnetic behavior in the PrNi1-xCuxAl compounds Author: Bc. Jan Fikáček Department: Department of Condensed Matter Physics Supervisor: Doc. Mgr. Pavel Javorský, Dr. Supervisor's e-mail address: javor@mag.mff.cuni.cz Abstract: In the present work we studied magnetic properties of the substituted PrNi1-xCuxAl series. A very interesting behavior had been reported in the previously studied systems with the same substitution, but with different rare earths contained, e.g. loss of long range order for certain concentrations of copper. We prepared polycrystalline samples of the PrNi1-xCuxAl (x = 0.1 - 0.9, 9 different stoichiometries) and measured them using X-ray diffraction, specific heat, magnetization and AC susceptibility. Additionally, powder neutron diffraction measurement on PrNi0.2Cu0.8Al sample was performed in ILL (Institut Laue Langevin) in Grenoble. Results of measurements on these compounds show on the presence of a long order in case of compounds with x = 0.1 - 0.4 below the ordering temperatures in the range of 3.4 - 5 K. Measurements of AC susceptibility and neutron diffraction revealed the loss of long range order in the rest of the series. In these compounds, the development of a spin glass state occurs below the temperatures between 3.4 and 4.5 K.
|
|
|
Physical phenomena in ytterbium- and cerium-based compounds
Fikáček, Jan ; Sechovský, Vladimír (advisor) ; Arnold, Zdeněk (referee) ; Andreev, Alexander (referee)
This work contains a study of CeRuSn, which undergoes two structural transitions at 290 K and 256 K both connected with large temperature hysteresis. During the transitions the lattice shrinks along the c axis. At low temperatures the compound orders antiferromagnetically below 2.8(1) K. A strong magnetocrystalline anisotropy is caused by very shortened Ce-Ru separations pointing approximately along the c axis. Due to a strong hybridization, two thirds of Cerium atoms are in a non integer valence state. For the first time synthesized single-crystals of YbPt2Si2 a Yb2Pt3Si5 show no magnetic ordering. A maximum, which is visible in the temperature dependences of magnetic susceptibility originate in thermal population of the magnetic Yb3+ state. Powered by TCPDF (www.tcpdf.org)
|
|
|
The development of magnetic behavior in the PrNi1-xCuxAl compounds
Fikáček, Jan
Title: The development of magnetic behavior in the PrNi1-xCuxAl compounds Author: Bc. Jan Fikáček Department: Department of Condensed Matter Physics Supervisor: Doc. Mgr. Pavel Javorský, Dr. Supervisor's e-mail address: javor@mag.mff.cuni.cz Abstract: In the present work we studied magnetic properties of the substituted PrNi1-xCuxAl series. A very interesting behavior had been reported in the previously studied systems with the same substitution, but with different rare earths contained, e.g. loss of long range order for certain concentrations of copper. We prepared polycrystalline samples of the PrNi1-xCuxAl (x = 0.1 - 0.9, 9 different stoichiometries) and measured them using X-ray diffraction, specific heat, magnetization and AC susceptibility. Additionally, powder neutron diffraction measurement on PrNi0.2Cu0.8Al sample was performed in ILL (Institut Laue Langevin) in Grenoble. Results of measurements on these compounds show on the presence of a long order in case of compounds with x = 0.1 - 0.4 below the ordering temperatures in the range of 3.4 - 5 K. Measurements of AC susceptibility and neutron diffraction revealed the loss of long range order in the rest of the series. In these compounds, the development of a spin glass state occurs below the temperatures between 3.4 and 4.5 K.
|
|
| |
|
|
The development of magnetic behavior in the PrNi1-xCuxAl compounds
Fikáček, Jan ; Prchal, Jiří (referee) ; Javorský, Pavel (advisor)
In the present work we studied magnetic properties of the substituted PrNi1-xCuxAl series. A very interesting behavior had been reported in the previously studied systems with the same substitution, but with different rare earths contained, e.g. loss of long range order for certain concentrations of copper. We prepared polycrystalline samples of the PrNi1-xCuxAl (x = 0.1 - 0.9, 9 different stoichiometries) and measured them using X-ray diffraction, specific heat, magnetization and AC susceptibility. Additionally, powder neutron diffraction measurement on PrNi0.2Cu0.8Al sample was performed in ILL (Institut Laue Langevin) in Grenoble. Results of measurements on these compounds show on the presence of a long order in case of compounds with x = 0.1 - 0.4 below the ordering temperatures in the range of 3.4 - 5 K. Measurements of AC susceptibility and neutron diffraction revealed the loss of long range order in the rest of the series. In these compounds, the development of a spin glass state occurs below the temperatures between 3.4 and 4.5 K.
|
guest ::
